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One of my favorites...
In the scene in Airplane where everyone is trying to calm down the hysterical woman, Nielsen (as the Dr.) takes over, shaking the woman and telling her to calm down, then slapping her. A nun comes by to relieve him, and he glances back to the woman, giving her one more slap for good measure before he leaves. For some reason, that extra slap just kills me.
Rest in Peace, Leslie.
Scott's note: I embedded the video for John, it's too fucking good not to, and it's Leslie's second slap that makes this sing: